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Both are nice neither one are the "hood" but I would choose South Loop Chicago only because I've actually been there and I think it's a nice area. I've only been to Atlanta a couple of times and never been to Midtown but I hear great things about it.
This is actually a really good comparison. I highly prefer South Loop Chi-town. It's just so much more aesthetically pleasing imo...even though I do really like Midtown ATL.
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