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I think that'd be really hard.
The Amtrak from Hartford to Penn Station takes 2-3 hours, and is 50-60 dollars each way.
The Greyhound from Hartford to Port Authority takes about 3 hours (often longer, I took it a bunch when I was in college and it was over an hour late about half the time), and is about 50$ round trip. I'm pretty sure those are the only two options, unless there's a daily commuting shuttle run by a limo company.
Since that's not including the time it'd take to travel from the station to home/work, I expect you'd be spending all your waking time traveling or working.
If you want regular access to NYC, or your partner works in the city, maybe try New Haven as a halfway point? That's just an hour into Hartford, and an hour-and-a-bit into NYC, with plenty of urban amenities.
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