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Probably the "Astoria" neighborhood in Queens, parts of Detroit.Out of actual incorporated cities, it's Tarpon Springs. Tarpon Springs is more German than Greek because most places in the US are German dominated, but few have a measurable Greek population.
I've heard that Tarpon Springs has the highest concentration of Greeks in the US, too. But even if it doesn't, I know I always love going there and eating fabulous Greek food along the sunny shores of the Gulf of Mexico and hearing a lot of Greek being spoken all around me.
There are large numbers of Greek/Greek heritage people in the Chicago and Detroit areas too. Tarpon Springs is a small town with a small Greek population.
Here's a map of the Greek diaspora in the U.S., based on the 2000 Census, and retrieved from wikipedia (sorry, there was no legend, so I don't know what to make of it. Just look at the pretty colors. Let's assume red means a lot of Greeks!):
Greektown in Chicago is awesome! That's where I've seen the most Greeks in one concentration.
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