I used to drive for Dartmouth Coach
I live in New London. The reason Dartmouth Coach only discharges in New London going northbound is they don't wish to be obligated to get off the highway if there are no passengers to drop. If it helps, they may be willing to take you from Hanover or Lebanon to New London if you call their office, (or drop in at their Lebanon station) and talk with the General Manager, David Fox, though as others have said, it's not their policy.
The ride share idea is worth pursuing. My wife works in Hanover but can't carpool because her work schedule can be irregular. Try Craigslist, Dartmouth College, or the Kearsarge Shopper, a weekly ad paper that gets mailed every Wednesday to every mailbox in about 10 area towns. Ads cost $20 or so, but it is very widely read around these parts.
HTH
Mark
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