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Honey Brook is the least rural as Downingtown is only a few miles away and it has a Wegman's, BJ's, chain restaurants. Further down 30 East you get lots of shopping in Exton.
That being said, Honey Brook is a rural and a hike to the city...like a 1.5 hour drive. We looked at homes there (very reasonable, very nice) but my 2 year old would scream after an hour in the car on the way to/from so that was enough for me.
We are living in Thorndale and love it as it is wooded but also plenty developed and only a few miles from the amenities mentioned above. There is also access to Septa Regional Rail and Amtrak close by.
For someone used to the city, you probably would want West Chester or Media as they have a walkable downtown area - Media puts you within 30 minutes of the city limits...
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