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... That kind of depends on what your interests are.
If you're into people, and into sort of "street culture," I might spend some time down by U Street between 12th and 16th Streets. You're not going to find street performers or anything, but it's a good crowd of a lot of different types of people walking around, some neat art and stickering on the sides of buildings (think mural-artist Shepherd Fairy), very hip culture. You can continue walking south from there and you'll be safe with your camera out, but I'd beware of walking north of that neighborhood (that'd be uphill).
You also might want to check out Eastern Market, which is accessible by Metro. If it's nice, there'll be a lot of people out, and if you're up to walking and get a street map, you might discover some interesting stuff. I don't spend a lot of time around there, but I recall there being an open air market on the weekends in the spring and summer that'd be cool.
If you like nature photography, you can visit the National Arboretum. And if you'll be striking out on a shooting-adventure soon, I believe the Cherry Blossom Festival begins now and will be happening for about two weeks. There's a parade and a Japanese street festival ... and then, of course, the blooming trees (which are quite beautiful). As a warning, there'll be large crowds.
Have fun!
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