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I know of a couple of farms for sale North of the (Frankonia) Notch in New Hampshire. I will be going up there for thanksgiving dinner with family. PM me and I'll get back to you.
I haven't read the replies yet, but Northeastern CT might suit you. It's very rural in parts. The area around UConn, for example, is on the edge of the so-called "Quiet Corner". It's as rural as you're going to find anywhere between Boston and Washington- woods, farms, and orchards. It's about 40 minutes to Hartford from here. If you go further east it gets more rural, but closer to Providence.
In the middle of nowhere, but pretty close to a lot of places.