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If you add townships quite a few pop in the Philly area but these are cities (but towns in the area have really small borders so no huge population by single municipality
Like these in the Philly area
Upper Darby 87K
Bensalem 62K
Lower Merion 58K
Abington 56K
Bristol 55K
Haverford 49K
Location: Chapel Hill, NC, formerly NoVA and Phila
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Not what you asked, but
Philadelphia contains the largest city of another state (Wilmington, DE) in its metropolitan area.
New York City does too with New Jersey's largest city of Newark.
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