You want to search for "white metal casting"
Low temp alloys can be cast in silicone molds, but they molds wear out quickly. With resin you might get 60 or 100 pulls from a mold (depending on the silicone chosen for the mold), I would guess with white metal you will get 10 or less - I've not tried casting white metal though - resin is plenty tricky enough!
This seems like a pretty good article, though I've only skimmed it:
Whitemetal Casting for Beginners – The Theory
This is a good one too, has decent pics.
Metal Casting
A good silicone and resin source I've used is Hobby Silicone in Los Angeles.
The only alloy for sale I've seen is pretty expensive. If you can do some home metallurgy and come up with a zinc alloy that will melt at 500 C or so, you can get zinc wheel weights from guys who cast bullets. They hate the zinc ones and will usually sell them cheap.
Depending on your intended use, you might be able to use straight wheel weight alloy - its lead and antimony. With adequate precautions, casting lead is safe (the bullet guys can tell you all about the precautions).