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How about Peterborough?! Are you looking at Waldorf schools? People from P'Boro go to both Monadnock Waldorf in Keene (active carpooling group) and to High Mowing /Pine Hill in Wilton. The other big private schools in the area are the Well School, Mountain Shadows (1-8), and the Dublin School (high school).
It's a really walkable, lively town and very much into "green." We had a big "Greenerborough" fair in the Spring and there are lots of exciting projects and resources for green building in the area. We're part of a green neighborhood project so I feel tapped into it more than your average person, but there does seem to be a lot going on here.