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I haven't been to all of them but I voted Gertrude St because it seemed to have a good balance between food/shopping/entertainment and I just liked the architecture/vibe a lot. I liked most of them though - Ackland St and Lygon St seemed to have great food, Chapel St shopping and I was on Smith St for a bit but I didn't get a proper chance to look around. I'd love to visit the rest sometime.