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Atlanta is currently the newest and largest, and is in the midst of a huge dolphin expansion right now. It's pretty impressive.
I also love the National Aquarium in Baltimore, Aquarium of the America's in Nola and the Chattanooga Aquarium (possibly the most underrated in the country).
Never been to the one in Monterey, but I've heard that it's fantastic.
I also enjoy the Tennessee Aquarium. I like how it sends you up an escalator to the top, and you move along a path that takes you through various exhibits from top to bottom. It also has a newer second building for saltwater habitats.
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